Environmental Life Cycle Implications of Using Bagasse- Deri
Contract No. DE-AC36-99-GO10337
November 2000 NREL/TP-580-28705
Environmental Life Cycle
Implications of Using Bagasse-
Derived Ethanol as a Gasoline
Oxygenate in Mumbai (Bombay)
Kiran L. Kadam
Prepared for the National Energy Technology Laboratory
Pittsburgh, Pennsylvania, USA and
USAID, New Delhi, India
National Renewable Energy Laboratory
1617 Cole Boulevard
Golden, Colorado 80401-3393
Contract No. DE-AC36-99-GO10337
November 2000 NREL/TP-580-28705
Environmental Life Cycle
Implications of Using Bagasse-
Derived Ethanol as a Gasoline
Oxygenate in Mumbai (Bombay)
Kiran L. Kadam
Prepared for the National Energy Technology Laboratory
Pittsburgh, Pennsylvania, USA and
USAID, New Delhi, India
Prepared under Task No. WG88.0101
National Renewable Energy Laboratory
1617 Cole Boulevard
Golden, Colorado 80401-3393
Contract No. DE-AC36-99-GO10337
NOTICE
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constitute or imply its endorsement, recommendation, or favoring by the United States government or any
agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect
those of the United States government or any agency thereof.
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Contract No. DE-AC36-99-GO10337
TABLE OF CONTENTS Acknowledgments____________________________________________________________vii
Executive Summary___________________________________________________________1
Background______________________________________________________________________1
Study Objective and Results________________________________________________________1
Next Phase of the Project___________________________________________________________2
1
2
3 Introduction_____________________________________________________________3 Project Scope____________________________________________________________3 Sugarcane and Sugar Production____________________________________________4
3.1
3.2
3.3 World Sugar Situation_______________________________________________________4 Sugarcane Production in India________________________________________________4 Sugar Industry in Maharashtra_______________________________________________4
Ethanol Capacity___________________________________________________________8
Bagasse Storage____________________________________________________________8
Related Research___________________________________________________________9
Study Objective____________________________________________________________9
Study Phases_______________________________________________________________9
Life Cycle Assessment Principles______________________________________________9
Methodology______________________________________________________________11 Functional Unit_________________________________________________________________11
Definition of System Boundaries___________________________________________________11
Interpretation: Life Cycle Impact Assessment_________________________________________12 4 Bioethanol Production in Maharashtra_______________________________________7 4.1 4.2 5 Life Cycle Assessment_____________________________________________________9 5.1 5.2 5.3 5.4 5.5 5.5.1 5.5.2
5.5.3
6 Scoping Options and Decisions_____________________________________________12
6.1 6.1.1
6.1.2
6.1.3
6.1.4
6.2.1
6.2.2 Project Parameters________________________________________________________13 General System Boundaries_______________________________________________________Environmental Issues Considered___________________________________________________Geographical Scope_____________________________________________________________Temporal Scope________________________________________________________________13 14 16 17 6.2 Product Parameters________________________________________________________18 Scenarios______________________________________________________________________18
Functional Unit_________________________________________________________________18
6.3
6.4 6.4.1 Process Parameters________________________________________________________19 LCA-Specific Parameters___________________________________________________20 Allocation Rules________________________________________________________________20
Contract No. DE-AC36-99-GO10337
6.5 Summary of Scoping Decisions and Approaches________________________________20
LCA Software_____________________________________________________________21
General Bagasse Data______________________________________________________21
Bagasse Burning___________________________________________________________25
Ethanol Production________________________________________________________25 Enzymatic Process______________________________________________________________26
Two-Stage Dilute Acid Process____________________________________________________28
Data Summary for Bagasse-to-Ethanol Processes______________________________________29 7 Life Cycle Modeling______________________________________________________21 7.1 7.2 7.3 7.4 7.4.1 7.4.2
7.4.3
7.5
7.6
7.7
7.8
7.9
7.10
7.11 Sulfuric Acid Production____________________________________________________29 Ammonia_________________________________________________________________30 Lime_____________________________________________________________________31 Electricity Production______________________________________________________31 Steam Production__________________________________________________________31 Gasoline System___________________________________________________________32 Gasoline and E10 Fuel Combustion___________________________________________32 7.11.1 Tailpipe Emissions______________________________________________________________32
7.11.2 Biomass versus Fossil Fuel CO2____________________________________________________33
8 Data Quality and Sources_________________________________________________34
8.1
8.2 Data Sources______________________________________________________________34 Data Quality______________________________________________________________35
Presentation of Results_____________________________________________________36
Explanation of Negative Flows_______________________________________________36
Hydrocarbon Emission_____________________________________________________36
Time-Space Implications of Emissions_________________________________________36
Life Cycle Energy Balance__________________________________________________36
LCI for Burning versus Diverting Bagasse to Ethanol: Enzyme Process____________38 Resource Depletion______________________________________________________________
Air Pollutants__________________________________________________________________
Waste Generation_______________________________________________________________
Energy Consumption and GHGs____________________________________________________40 40 40 40
49
49
49 49 9 Results and Discussion____________________________________________________36 9.1 9.2 9.3 9.4 9.5 9.6 9.6.1 9.6.2 9.6.3 9.6.4 9.7.1 9.7.2 9.7.3 9.7.4
9.8.1 9.8.2
9.8.3 9.7 LCI for Burning versus Diverting Bagasse to Ethanol: Dilute Acid Process__________48 Resource Depletion______________________________________________________________Air Pollutants__________________________________________________________________Waste Generation_______________________________________________________________Energy Consumption and GHGs____________________________________________________9.8 LCIA for Burning versus Diverting Bagasse to Ethanol__________________________49 Greenhouse Potential____________________________________________________________50 Natural Resource Depletion Potential________________________________________________50
Air Acidification Potential________________________________________________________51
Contract No. DE-AC36-99-GO10337
9.8.4
9.8.5
9.8.6 9.8.7 Eutrophication Potential__________________________________________________________Human Toxicity Potential_________________________________________________________Air Odor Potential_______________________________________________________________
Maximum Incremental Reactivity Potential___________________________________________51 54 54 54
10
11 Conclusion___________________________________________________________56 Next Phase of the Project________________________________________________57
List of Acronyms and Abbreviations_____________________________________________59
References__________________________________________________________________60
Appendix A: Project Review___________________________________________________63
Appendix B: Impact Assessment________________________________________________64
Background_____________________________________________________________________64
Overview of Life Cycle Impact Assessment Indices_____________________________________66 Greenhouse Potential____________________________________________________________________
Acidification Potential___________________________________________________________________
Eutrophication Potential_________________________________________________________________
Natural Resources Depletion Index_________________________________________________________
Human Toxicity Index___________________________________________________________________
Stratospheric Ozone Depletion Index_______________________________________________________66 66 67 68 70 74
Index Calculation________________________________________________________________74 Odor Index____________________________________________________________________________76
Appendix C: List of Alcohol Manufacturers in Maharashtra_________________________78
Contract No. DE-AC36-99-GO10337
vLIST OF TABLES
Table 1. India’s leading sugarcane-producing states_________________________________________________4
Table 2. Comparison of Maharashtra state and Indian national sugar statistics____________________________6
Table 3. Number of sugar mills in India by cane crushing capacity______________________________________6
Table 4. Sugar factories in Maharashtra by geographical region_______________________________________7
Table 5. Data for VSSK Ltd.’s sugar mill in Sangli, Maharashtra_______________________________________7
Table 6. Environmental inventory flows considered_________________________________________________16
Table 7. Equivalency between current gasoline and E10 blend________________________________________18
Table 8. Summary of scoping decisions and approaches_____________________________________________21
Table 9. Proximate chemical composition of bagasse produced in Florida and Hawaii (oven-dry basis)_______22
Table 10. Proximate chemical composition of commercially baled sugarcane bagasse (oven-dry basis)_______23
Table 11. Calorific value and the elemental analysis for bagasse______________________________________24
Table 12. Recent data on bagasse composition____________________________________________________24
Table 13. Changes in bagasse composition due to storage____________________________________________24
Table 14. Data summary for bagasse-to-ethanol processes___________________________________________30
Table 15. Combustion-related properties of green feedstock and ligneous residues________________________30
Table 16. Overall emissions for current gasoline and E10 blend_______________________________________32
Table 17. Overview of change in emissions from low-level and high-level ethanol blends___________________33
Table 18. Apportioned emissions for E10 Blend____________________________________________________34
Table 19. Data sources and quality_____________________________________________________________35
Table 20. Explanation of negative flows__________________________________________________________37
Table 21. Life cycle inventory for burning versus perting bagasse to ethanol: Summary for enzyme process___39
Table 22. Natural gas consumption and CODs for key modules_______________________________________39
Table 23. Life cycle inventory for burning versus perting bagasse to ethanol: Summary for dilute acid process_48
Table 24. Life cycle impact assessment for burning versus perting bagasse to ethanol: Summary for enzyme
process___________________________________________________________________________________50
Table 25. Life cycle impact assessment for burning versus perting bagasse to ethanol: Summary for dilute acid
process___________________________________________________________________________________51
Table 26. Ozone-forming potential of selected compounds___________________________________________54
Table 27. Greenhouse gas potential factors_______________________________________________________66
Table 28. Acidification potential reactions________________________________________________________67
Table 29. Eutrophication potential factors________________________________________________________68
Contract No. DE-AC36-99-GO10337
LIST OF FIGURES
Figure 1. Geographical distribution of sugarcane production in India........................................................................5
Figure 2. Schematic representation of extending system boundaries.........................................................................10
Figure 3. Elements of the scoping phase for life cycle analysis..................................................................................13 Figure 4. General system boundaries for the comparison of burning of excess bagasse versus its persion to ethanol
production...................................................................................................................................................................14
Figure 5. Energy and mass equivalency between current and future scenarios in the context of the functional unit.19
Figure 6. Enzymatic process flow diagram.................................................................................................................26
Figure 7: Two-stage dilute-acid process flow diagram..............................................................................................28
Figure 8. Comparison of burning versus perting bagasse to ethanol: Coal usage..................................................41 Figure 9. Comparison of burning versus perting bagasse to ethanol: Natural gas usage.......................................41
Figure 10. Comparison of burning versus perting bagasse to ethanol: Crude oil usage........................................42
Figure 11. Comparison of burning versus perting bagasse to ethanol: Water usage..............................................42
Figure 12. Comparison of burning versus perting bagasse to ethanol: Carbon monoxide emissions.....................43
Figure 13. Comparison of burning versus perting bagasse to ethanol: Hydrocarbon (except methane) emissions.43
Figure 14. Comparison of burning versus perting bagasse to ethanol: Sulfur oxides (SOx as SO2) emissions.......44 Figure 15. Comparison of burning versus perting bagasse to ethanol: Nitrogen oxides (NOx as NO2) emissions..44
Figure 16. Comparison of burning versus perting bagasse to ethanol: Particulate matter (unspecified) emissions.
....................................................................................................................................................................................45
Figure 17. Comparison of burning versus perting bagasse to ethanol: Lead emissions.........................................45
Figure 18. Comparison of burning versus perting bagasse to ethanol: Fossil CO2 emissions................................46 Figure 19. Comparison of burning versus perting bagasse to ethanol: Methane emissions...................................46
Figure 20. Comparison of burning versus perting bagasse to ethanol: Process energy usage...............................47
Figure 21. Comparison of burning versus perting bagasse to ethanol: Nonrenewable energy usage.....................47
Figure 22. Comparison of burning versus perting bagasse to ethanol: Greenhouse effect potential......................52
Figure 23. Comparison of burning versus perting bagasse to ethanol: Depletion of non-renewable resources.....52
Figure 24. Comparison of burning versus perting bagasse to ethanol: Air acidification potential.........................53 Figure 25. Comparison of burning versus perting bagasse to ethanol: Eutrophication potential...........................53
Figure 26. Comparison of burning versus perting bagasse to ethanol: Human toxicity potential..........................55
Figure 27. Comparison of burning versus perting bagasse to ethanol: Air odor potential.....................................55
Figure 28. Comparison of burning versus perting bagasse to ethanol: EPA-Maximum incremental reactivity
potential......................................................................................................................................................................56
Figure 29. Life cycle impact assessment framework...................................................................................................65
Contract No. DE-AC36-99-GO10337
ACKNOWLEDGMENTS
This work was supported by the National Energy Technology Laboratory, Pittsburgh, PA, USA,
and the U.S. Agency for International Development (USAID), New Delhi, India. The author
wishes to thank these entities for financing the study and members of the Review Committee
(see Appendix A) for their thoughtful review of this report and many useful comments and
suggestions. Vince Camobreco of Ecobalance Inc. and John Sheehan of NREL deserve a special
mention for their help throughout this project.
Contract No. DE-AC36-99-GO10337
EXECUTIVE SUMMARY
Background
Bagasse is the fibrous residue generated during sugar production and can be a desirable
feedstock for fuel ethanol production. About 15%–25% of the bagasse is left after satisfying the
mills’ energy requirements, and this excess bagasse can be used in a bioconvesion process to
make ethanol. It is estimated that a 23 million L/yr (~6 million gal/yr) ethanol facility is feasible
by combining excess bagasse from three sugar mills in Maharashtra state. The annual gasoline
consumption in Mumbai is estimated to be 400–500 million L, and the plant could supply about
half of the ethanol demand, assuming that all gasoline is sold as an E10 fuel, a blend of 90%
gasoline and 10% ethanol by volume.
This study discusses the potential benefits of using bagasse-derived fuel ethanol in India. This
strategy is pertinent to the Indian scene because it can: 1) reduce the net emissions of carbon
dioxide, 2) improve air quality in major metropolitan areas such as Mumbai when used as an
oxygenate additive to gasoline, 3) spur rural economic development, and 4) improve the
country’s energy security by reducing its reliance on foreign oil and associated risks.
Study Objective and Results
The study objective is to conduct a life cycle assessment (LCA) to quantify the environmental
benefits of using bagasse-derived ethanol as a gasoline oxygenate in Mumbai. The LCA results
would serve as a basis for deploying bagasse-to-ethanol production in Maharashtra, because
positive environmental benefits—both in terms of local air quality and climate change—align
with USAID’s mission and objectives.
The LCA performed in this study demonstrates the potentially significant benefits of using
ethanol derived from bagasse in Maharashtra. The overall results revealed a fundamental
difference between Scenario 1 (burning excess bagasse as a disposal option) and Scenario 2
(conversion to ethanol) in terms of energy derived from renewable sources and the concomitant
benefits of reduced greenhouse gas emissions. In particular, lower net values for the ethanol
scenario were observed for the following:
Carbon monoxide
Hydrocarbons (except methane)
SOx and NOx
Particulates
Carbon dioxide and methane
Fossil energy consumption
Hence, implementing the ethanol scenario would reduce air emissions and fossil energy
consumption. Reduced carbon dioxide and methane emissions, although not regulated or
mandated by state or national laws, are also desirable attributes. The lower greenhouse potential
of Scenario 2 can be important if greenhouse gas trading is possible, or in the case of Joint
Contract No. DE-AC36-99-GO10337
Implementation because India is a developing country. Additional drivers are the lower values
observed for the following six impact assessment categories for the ethanol scenario, when
compared to the burning scenario:
Greenhouse potential
Depletion of natural resources
Air acidification potential
Eutrophication potential
Human toxicity potential
Air odor potential
Hence, the ethanol scenario distinguishes itself by demonstrating lower burdens than the burning
scenario for key environmental criteria, both regulated and unregulated.
Next Phase of the Project
The next phase should address how to deploy this option in India by capitalizing on the
environmental benefits of perting the excess bagasse to ethanol production. The action plan
would involve institutional and stakeholder networking and would address deployment this
technology with the help of relevant parties in India, from both the public and private sectors.
Early this year, India’s Minister of Petroleum and Natural Gas approved the use of ethanol as a
fuel/additive. During his recent trip to India, President Clinton signed a joint statement on
cooperation between India and the United States in the areas of energy and environment; the
statement has language about Clean Development Mechanism as specified under the Kyoto
Protocol. Hence, these recent developments in India portend a fertile ground for deploying the
bioethanol option in India.
Contract No. DE-AC36-99-GO10337
1 INTRODUCTION
Worldwide economic development will lead to increased emissions of greenhouse gases (GHGs)
well into the next century. Developing countries like India and China are expected to be major
contributors to atmospheric carbon dioxide (CO2) build-up and are potential targets for the
deployment of biomass-based technologies, given the large amounts of biomass available within
their borders.
India is the world’s sixth largest and second fastest growing producer of greenhouse gases. In
1992, India’s carbon emissions were 177 Mt (million metric tons), the third largest among non-
OECD (Organization for Economic Cooperation and Development) countries. Fossil fuel energy
consumption was about 7.5 quadrillion Btu, 15% of which was attributable to the transportation
sector. About the same fraction of the total carbon emissions was associated with the
transportation sector. Hence, significant carbon emissions arise from the use of fossil fuels for
transportation in India. Vehicular emissions also contribute to local air pollution. Delhi, Mumbai
(formerly Bombay), and Chennai (formerly Madras) are three of the world’s ten most polluted
cities. For the specific case of Mumbai, the National Environmental Engineering Research
Institute in Nagpur, India, estimates that motor vehicles will contribute nearly 90% of the
255,000 t/yr of carbon monoxide (CO) emissions. Oxygenating the gasoline with ethanol can
reduce CO emissions.
This report discusses the potential benefits of using bagasse-derived fuel ethanol, a strategy that
is relevant to India, as it can: 1) reduce the net emissions of CO2 into the atmosphere, 2) improve
air quality in major urban centers such as Mumbai when used as either a 10% (by volume)
oxygenate additive to gasoline (short-term) or as an alternative to gasoline (long-term), 3)
provide rural economic development, and 4) improve the country’s energy security by reducing
its exposure to risks associated with foreign oil.
2 PROJECT SCOPE
The primary objective is to conduct a life cycle assessment (LCA) to quantify the environmental
benefits of using bagasse-derived ethanol as a gasoline oxygenate in Mumbai. The LCA results
will serve as a basis for deploying bagasse-to-ethanol production in Maharashtra, because
positive environmental benefits—both in terms of local air quality and climate change—align
with USAID’s (U.S, Agency for International Development) mission and objectives. A brief
discussion is also provided on how Joint Implementation (JI) and Clean Development
Mechanism (CDM) initiatives and emissions trading, opportunities available to developing
countries under the United Nations Framework Convention on Climate Change, can be used to
help deploy bagasse-to-ethanol production India.
Contract No. DE-AC36-99-GO10337
3 SUGARCANE AND SUGAR PRODUCTION
3.1 World Sugar Situation
Brazil and India are the world’s two largest sugarcane (Saccharum officinarum) growers with
production of 300 and 285 Mt/yr, respectively (Lower and Barros 1999; Singh 2000). These two
countries are also expected to account for nearly 75% of the future increase in sugarcane
production. World sugar consumption in 1999–2000 is estimated at 131.3 Mt, up 2% from the
previous year’s level, with Brazil and India contributing 19.0 and 17.9 Mt, respectively (World
Bank 2000).
3.2 Sugarcane Production in India
As demonstrated in Table 1, India’s leading sugarcane-producing states are Uttar Pradesh,
Maharashtra, and Tamil Nadu, together accounting for about 70% of the national output (Smouse
et al. 1998; Deccan Herald 1999). Although the focus of this study is Maharashtra, similar
ethanol-producing facilities are possible in Uttar Pradesh and Tamil Nadu, and these could
provide ethanol for an E10 blend, respectively, for Delhi and Chennai, the other two Indian cities
to have the dubious distinction of being on the list of the world’s 10 most polluted cities. The
geographical distribution of this important crop for the entire country is shown in Figure 1
(USDA 1998).
Table 1. India’s leading sugarcane-producing states 1998-1999a
% of Production, % of Production, % of
Mt Total Mt Total Mt Total
b NAbTamil b NAb
Estimates.
Not available. b a
3.3 Sugar Industry in Maharashtra
Maharashtra State is a leader in both agriculture and industrial growth in India. As shown in
Table 1, Maharashtra is the second largest sugarcane producing state in India. Typical sugar
industry statistics for Maharashtra are shown below (REPSO 1998).
Annual average cane production: 40–45 Mt
Average sugar recovery: 11.11 Mt
Number of sugar mills: 109 (cooperatives)
A comparison of Maharashtra state with the country as a whole, in terms of key industry
parameters for the last 5 years, is presented in Table 2 (Maharashtra State Govt. 1998). Table 3
Contract No. DE-AC36-99-GO10337
indicates that Maharashtra ranks second in India, based on the number of cane sugar mills
(Maharashtra State Govt. 1998). However, in sugar production, it ranks first and surpasses even
Uttar Pradesh, due to its high yield of sugar per t of cane. Since 1987, a minimum capacity of
2,500 t crushed per day (TPD) has been imposed for new mills, and incentives are in place to
encourage expansion of existing mills to 5,000 TPD (Winrock International 1993). Maharashtra
has 12 and 6 mills with crushing capacities of >3,500 TPD and >5,000 TPD, respectively.
The southern and western Maharashtra regions have a greater share of cooperative sugar
factories in the state. Table 4 offers regional distribution of sugar factories in Maharashtra
(Maharashtra State Govt. 1998).
Figure 1. Geographical distribution of sugarcane production in India.
Contract No. DE-AC36-99-GO10337
Table 2. Comparison of Maharashtra state and Indian national sugar statistics
cultivation,
‘000 ha
production, Mt
Crushing
capacity,
Mt
No. of sugar
mills
Average
recovery, %
cane
Sugar
production, Mt Maharashtra Statea1993-1994-1995-1996-1993-1994-1995-1996-1994 19951996 1997 1994 1995 19961997 (10%) (14%)(14%) (12%) (12%) (16%)(17%) (15%) 24.68 45.9951.47 31.01 130.38 (25%) (31%)(30%) (24%) 97 107109 105 412 (25%) (26%)(26%) (26%) 9.429.90 2.75 (28%) 5.02(34%)5.39 (33%) 3.44 (27%) 12.90
a% numbers in parentheses represent Maharashtra’s contribution to the national statistics.
Table 3. Number of sugar mills in India by cane crushing capacity
Total
Number
of Mills
Number of Mills at Specified Capacities
Uttar Pradesh 36 13 43 7 12 111
17 35 12 109
Andhra Pradesh 20 3 9 1 3 36
Tamil Nadu 5 6 19 2 2 34
7 4 31
10 3 0 29
1 6 2 19
2 11 1 19
2 3 1 11
State TPD <1250 TPD 1250–2500 TPD 2500–3500 TPD 3500–5000 TPD >5000
Contract No. DE-AC36-99-GO10337
Table 4. Sugar factories in Maharashtra by geographical region
Geographical Region Number of Sugar Installed Capacity, Factories TPD
Total cooperatives 81 209,650
South and west 78 204,600
Central 27 51,250
Eastern 19 21,250
Table 5 lists data for Vasantdada Shetkari Sakhar Karkhana Ltd.’s (VSSK) sugar mill in Sangli,
Maharashtra (Winrock International 1993; Smouse et al. 1998). The cane-crushing capacity at
VSSK can be expanded to 7,500 TPD; however, mill management does not plan to expand
beyond 6,000 TPD. This mill is considered as a typical candidate mill pertaining to ethanol
production.
Table 5. Data for VSSK Ltd.’s sugar mill in Sangli, Maharashtra Parameter Value
Mill capacity, TPD 5000
Cane crushed, t/year 924,048
Crop duration, days/year 200
Average cane crushing rate, TPD 4,972
Downtime, % of milling season 19.4
Fiber, % of cane 13.7
Bagasse, % of cane 30.8
Moisture, % of bagasse 50.6
Bagasse produced, t 284,422
4 BIOETHANOL PRODUCTION IN MAHARASHTRA
Bagasse is the fibrous residue left after extraction of sugar from the cane and can be a good
feedstock for bioethanol (i.e., biomass-derived ethanol) production. Bagasse is preferably used
by the sugar mills for steam and power generation to satisfy internal needs; however, about 15%-
25% of the bagasse is left after satisfying the mills’ energy requirements, and this excess is not
burned in the mill boilers. (Steam consumption in Indian sugar mills is as high as 50-55% on
cane compared to 40% in Hawaii. With improvements in or replacement of existing boilers, the
excess bagasse figure could be higher.)
A bagasse-based ethanol project is in the planning/development stage in the United States. BC
International (BCI) is adapting a non-operational molasses-to-ethanol plant in Jennings,
Louisiana, to process local agricultural residue (USDOE 1998). This is a first stand-alone,
commercial, biomass-to-ethanol plant and is expected to produce about 75 million L/yr (20
million gal) of ethanol a year from sugarcane bagasse and rice hulls as feedstock. This project is
proceeding toward commercialization, and being an industrial-scale demonstration of the
biomass-to-ethanol technology, it can be used as a model for a plant in Maharashtra. Such an
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